Magnetic structure, phase diagram, and a new type of spin-flop transition dominated by higher order interaction in a localized 5f system U3Pd20Si6.

نویسندگان

  • Y Koike
  • N Metoki
  • Y Haga
  • K A McEwen
  • M Kohgi
  • R Yamamoto
  • N Aso
  • N Tateiwa
  • T Komatsubara
  • N Kimura
  • H Aoki
چکیده

The magnetic structure of the localized-5f uranium intermetallic compound U3Pd20Si6 has been determined by means of a neutron diffraction experiment. Our data demonstrate that this compound has a collinear coupling of the sublattice ordering of the uranium spins on the 4a and 8c sites. We conclude that higher-order exchange and/or quadrupole interactions are necessary to stabilize this unique collinear structure. We discovered a new type of spin-flop transition against the uniaxial anisotropy induced by this collinear coupling.

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عنوان ژورنال:
  • Physical review letters

دوره 89 7  شماره 

صفحات  -

تاریخ انتشار 2002